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Open the Excellentable in edit mode and go to "Format" Tab
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Select the cell/cells to align in Left, Center or Right then click "Justify Select" drop down button
Left: Click Left Align button
Center: Click Center Align button
Right: Click Right Align button
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Select the cell/cells to align in Top, Middle or Bottom then click "Vertical Align" drop down button
Top: Click Top button
Middle: Click Middle button
Bottom: Click Bottom button